Gamma Dose Rates at Rongelap Atoll, 1954-1963

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GAMMA DOSE RATES AT RONGELAP ATOLL, 1954-1963 Laboratory of Radiation Biology University of Washington UNITED STATES ATOMIC ENERGY COMMISSION l DIVISION OF TECHNICAL INFORMATION

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This repmt was prepared as an account of Government sponsored work. Neither the United StateB, nor the Commimion, nor any person acting on behalf of the Commission: A. Makes any warranty or representation, expressed or implied, with respect to the accuracy, completeness, or usefulness of the information contained in tide report, or that the use of any information, apparatua, method, or process disclosed In this report may not infringe privately owned rightn; or B. Assumes any liabilities with respect to the use of, or for damages resulting from the use of any information, apparatus, methed, or process disclosod in this report. An used in the above, “peraon acting on behalf of the Commi88ion” includes IMY employee or contractor of the Commission, or employee of euch contracted, to the extent that such employee or contractor of the Commlenion, or employee of such contractor prepares, disseminates, or provldea access to, any information pursuant to his employment or contract with the Commission, or his employment with euch contractor. This reporthas been reproduceddirectlyfrom thebest

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BIOLOGY AND MEDICINE (TID-45011) GAMMA DOSE ~TES AT RONGELAP ATOLL, 1954-1963 Laboratory of Radiation Biology University of Washington Work performed under Contract AT(45-1)1385 with the United States Atomic Energy Commission.

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GAMMA DOSE ~TES AT RONGEIJU? ATOLL, 1954-1963 Rongelap Atoll was contaminated with fallout from a thermonuclear device on March 1, 1954. Gamma-dose rates on D + 1 ranged from 3.5 r/hr to 35 r/hr. Until 1959 the decline of gamma-dose rates measured in the field followed the theoretical decay of mixed fission products from U235 calculated by Miller and reduction of gamma dose rates to approximately half levels in 1959-63 probably reflects the downward movement of the fallout had little effect on gamma dose rates except in the intertidal zone. It is concluded that predicted gamma dose rates from fallout based on the theoretical decay curv@ of radionuclides from fission of U would tend to be equal to or greater than actual levels.

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GAMMA DOSE RATES AT RONGELAP ATOLL, 1954-1963 Rongelap Atoll, Marshall Islands, was accidentally contaminated on March 1, 1954 with radioactive fallout from a thermonuclear device detonated at Bikini Atoll some 80 miles to the west. Eighty-two natives residing on Rongelap Island were evacuated and repatriated in June 1957. The atoll, its inhabitants and its economy have been briefly characterized . The decline of gamma dose rates resulting from the fallout is discussed in this report. Gamma dose rates at Rongelap Atoll on D + 1 (time of detonation plus one day) were estimated to be 3.5 r per hour at the inhabited islet of Rongelap in the south and 35 r per hour at unhhabited Lomuilal islet in the northern part of polations of measurements made two days after initial fallout . The subsequent decline of gamma meter readings taken three feet and Kabelle islets, is compared dose rates, based on survey above the ground at Rongelap

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in Figs. 2 and 3. The theoretical cue is based on fission products from slow neutron fission and the assumptions that there is no fractionation and that the radionuclides are distributed over an infinite plane, while at Rongelap measurable amounts of activity remained on the trees. The actual measurements fit closely to the theoretical decay curve for Rongelap islet and at least for the first four years after fallout at Kabelle islet in spite of the assumptions made in determining the theoretical curve and the variability of the field measurements. The measurements on one small islet may vary by a factor of more than three, even when the identical instrument is used by the same person. $ Decline folhwinq first storm About two weeks after initial contamination there was a storm with heavy rain, and a subsequent reduction in gamma dose rate somewhat greater than would have been expected on Fallout in 1956 and 1958 The rises in gamma dose rates in 1956 and 1958 were due to operations Redwing and Hardtack. Even though there was a measurable amount of contamination, as was seen by the shortlived radionuclides present and by following the beta decay rates in plants collected in 1958, the total contributim was

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a fraction of one per cent of the fallout deposited in 1954. Therefore the Redwing and Hardtack fallout are ins~gnificmt when considering the long-range picture. Selection of areas and reproducibility of repeated measurements In March 1958, stakes were set out in various parts of Rongelap islet i.nan attempt to provide a means of repeating measurements at identical locations. Stakes proved to be unsatisfactory since they only served to attract the curious, which resulted in trampling and disturbance of the areas ande in some cases removal of the stakes. A practical solution to this problem was to select general areas within which measurements were to be taken. These areas were located with relation to pathways, roads, buildings, and measured distances from landmarks . In each general area measurements were taken over different types of vegetation, soil, the pathways themselves, over litter, and under Pandanus trees and other tall plants. In August 1958, the set of measurements was repeated three times at Rongelap islet and twice at both Eniaetok and Kabelle islets. At Rongelap islet the average for each set of readings ranged from 0.046 to 0.067 rnr/hr. At Eni.aetok the range of the average readings was 0.073 to 0.079 mr/hr and at Kabelle islet,

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Local differences in dose rates at three feet The highest levels measured were generally under trees, particularly under Pandanus trees where litter had accumulated. The highest levels at Rongelap islet in 1955 were measured in the remaining palm-frond huts where fallout remained trapped in the roof and the wall thatching. Readings the floor were lower than those at three feet and readings close to the walls and There were relatively high soil algae were abundant. one inch abae above the ground highest of all. algae form a crust roughly one centimeter thick and retain most of the radionuclides from Return to baclwround level The return to background level,< 0.02 ~fir, occurred would be expected, in the intertidal zone, except small areas of beach rock cavered with a film of algae. ZO.02 mr/k were measured in July, 1957 in the intertidal zones at Kabelle and Rongelap islets and in the newly constructed village on Rongelap islet. Construction of the village entailed the removal of the thatched huts and bulldozing of a considerable part of the area.

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Local differences in dose rates at one inch Survey meter readings were also taken at one inch above t ground with the beta shield both open and closed. There was n apparent correlation between these readings and the gamma dose rate readings at three feet, except in a very general way, but such readings were useful in selecting areas from which to sam and indicated local distribution of the activity. For example when measurements were made one inch over the ground with the shield open in 1959, the levels were higher after the litter was re”moved from the soil and there were markedly higher le;el of activity over areas covered with soil algae than over bare sand. Attempts also were made with a survey meter to determin local differences in activity in trees. This was unsuccessful since the general levels of activity masked local effects with the trees, even though laboratory analyses showed that the activity in lichens and mosses collected from the bark was several times higher than in the bare portions of the trees. The use of survey meters to determine the vertical distributio of activity in soil pits was impracticable due to the high bac ground levels from surrounding contamination and the fact that the bulk of the radioactivity was in the surface inch or less

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In September 1959, film badges sealed against moisture were exposed at Rongelap and Kabelle islets to measure gamma doses in different areas. The badges were provided and set out by Radiation Safety personnel at the Pacific Proving Ground. The limit of detection was an accumulated dose of 10 mr. Three badges were placed at each location, one suspended by strings three feet above the ground and away from tree trunks, one three feet above the ground attached to a tree, and one on the ground. Gamma dose rates measured with a smey meter at each location indicated that the accumulated dose in 69 out of 116 film badges would be in excess of 10 mr, but less than 20 mr. The results were, however, negative for all badges. The discrepancy between the doses calculated from the survey meter measurements and those obtained with film badges may be explained by differences in of the two methods to the gamma energies present in Calibration was based on a than on actual fallout material. This invalidate the decline curves in Figs. retical cu~e (solid Mne) is based on radium standard rather discrepancy does not 2 and 3 since the theometer similar to those used for the various measurements made. However, the discrepancy does point out that while relative levels of activity can be determined accurately by any one type of measurenu?nt, absolute values depend on calibration with

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rwioac sources having the same range and proportion of energieb the fallout material. Decline and fallout composition has turned out in practice at Rongelap Atoll that when number of survey meter readings are taken and these are averaged, a pattern of decline of gamma-dose rates consistent with the theoretical decay for mixed fission products emerges. This is true even though the theoretical curve is based on the de:ay of mixed fission products from U distributed uniformly over an infinite plane and disregards differences in both the composition and distribution of fallout radionuclides in the actual field situation. The fallout at Rongelap consisted of mixed fission products and neutron-induced radionuclides from a thermonuclear device. The induced activities contributing to the gamma activity are of shorter half life than the long-lived fission product, 30-year Cs . It therefore might have been expected that the early decline in gamma dose rates at Rongelap would have been more rapid than the theoretical decay of mixed fission products alone. As the art of producing thermonuclear devices progresses the fission yield per kiloton will decrease. l’here.will be a a higher proportion of induced radionuclides to fission products

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an..the - line of gamma dose rates will be more rapid. Therefore, ir. future, long-range predictions of residual gamma dose rates based on the Rong@lap experience would be likely to yield higher values than would actually occur. Fractionation of fallout In addition to the differences in composition of fallout from different devices and variations in measurements there is fractionation of the radionuclides, a change in species compositkn with time or distance from origin. The various factors involved in fractionation are discussed in detail in the Congressional and with specific reference to the March 1: Redistribution of fallout Reduction of gamma-dose rate levels due to redistribution of fallout possibly occurred during the first storm after fallout (Dunning, 1957) , but thereafter redistribution had very little effe& on the gamma dose rates during the first four years after fallout. The exception, of course, is the relatively rapid decline of radioactivity in the intertidal zone. Such rapid decline would also be anticipated in areas in which there is heavy erosion. An example is the man-made erosion by bulldozers in the village area at Rongelap. The reduction of gamma dose rates following the storm could have been due to the washing of fallout material

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from the leaves of the vegetation and perhaps also to some shielding effect by additional moisture in the soil. It was certainly not due to rapid vertical movement of material in the soil. Analysis of soil leachates and soil cores shows that vertical movement of radionuclides in atoll soils is very slow. For example, cores taken in immature soils in tained 90 per cent of the activity in the top the reduction of gamma-dose rates to predicted levels in 1959-63 probably soil . Cesium-137 and Sb are very slowly leached in the atoll , and Mn tend to remain at the surface (1,6,7)l Although the gamma-dose rate values at Rongelap islet in 1959-63 fall on the theoretical curve, it appears that the levels due to the 1954 fallout have fallen below values predicted by the theoretical curve here also. Since the theoretical curve had reached background levels by 1959 it would be expected that the sum of ganuna-dose rates due to the fallaut and due to background would be approximately twice background. The Rongelap experience has shown that the decline of gamma dose rates can be approximated from the decay tune for

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~235 fission products in a local or intermediate fallout situation. As instrumentation, techniques of calibration and the predictability of the radionuclide spectrum from nuclear devices continue to improve, so will the usefulness of gamma-dose rate measurements for predicting the decline of gamna~ose rates. Practical& speaking, the reliability of such measurements will depend upon the experience and judgement of the individuals making the measurements, the variety of environmental situations and the time available for making such measurements. reliability is further substantiated by the fact that of specific radfonuclides in the various land organisms at d}fferent islands were roughly correlated with the gamma dose rates. Errors in predicted levels will tend to be conservative, i.e., higher than actual levels. It would be useful in any future operations to have available known mixtures of radionuclides simulating the fallout particular device, or better, a sample of the raw fallout material collected at each site to be studied. This mixture could then be used to calibrate instruments, film badges and chemical dosimeters as time went on and as the spectrum of ganuna-energies changed. Comparison of the decay of

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gama-dose rates from the mixture, with decline of gamma-dose rates in the field, would give a more accurate indication of the overall effect of the redistribution of radionuclides on the gamna dose rates.

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Gamma Dose Rates \ operation Operation on Rongelap Island 0 University of Washington \\ fission products as measure o ‘\ radiac at 3 feet above an \ Days after March 1,1954 and Marchl of each year indicated Fig. 2. Decline of ~ Dose Rates at Rongolap Island.

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Gamma Dose Rates on products as measured by the feet above an infinite plane Days after March 1,1954 and March 1 of each year indicated Fig. 3. Decline of Gaxmna Dose Rates at Kabelle Islet.

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1. E.E. Held, Qualitative Distribution of Radionuclides at Rongelap Atoll. In Radioecolm , Schultz and Klement (Editors), Reinhold Pub. Corp. and the M@rican Institute of Biological Sciences~ New York (1963). 2. G.M. Dunning (Editor), Radioactive Contamination of Certain Jkeas in the Pacific Ocean from Nuclear Tests. U.S. Atomic 3. C.F. Miller and P. Loeb, Ionization Rate and Photon Pulse Rate of Fission Products from Slow Neutron Fission of U . 4. S. Glasstone (Editor), The Effects of Nuclear Weapons. …